The Dark Lord knew it would give him a body and immortal life.
The Dark Lord didn’t seem particularly concerned about whether the Elixir of Life would remove the curse that killing a unicorn and drinking its blood carries, but he wanted the Philosopher’s Stone for two reasons - to assure himself immortal life and to regain a body.
“But my plan failed. I did not manage to steal the Philosopher’s Stone. I was not to be assured immortal life. I was thwarted … thwarted, once again, by Harry Potter …”
- Harry Potter and the Goblet of Fire, Chapter 33 (The Death Eaters)
Though the Dark Lord was willing to change his plan once he knew he couldn’t get the Stone, he’d wanted it to restore himself to a hopefully stronger body.
“There was no hope of stealing the Philosopher’s Stone any more, for I knew that Dumbledore would have seen to it that it was destroyed. But I was willing to embrace mortal life again, before chasing immortal.”
- Harry Potter and the Goblet of Fire, Chapter 33 (The Death Eaters)
Also, Dumbledore said that the Dark Lord wanted it to regain a body, though he said the Dark Lord wouldn’t want to remain dependent on the Elixir of Life for too long.
“Of course he was prepared to drink it if it would take him out of the horrible part-life to which he was condemned after attacking you, but only to regain a body.”
- Harry Potter and the Half-Blood Prince, Chapter 23 (Horcruxes)
It’s made clear why the Dark Lord wanted the Philosopher’s Stone, but removing the unicorn blood curse didn’t seem to be anywhere among his considerations.